You can’t run the official Definitive Edition (the one from 2021 on PC/consoles) directly on PPSSPP. That version uses Unreal Engine 4 and is too heavy for PSP emulation.
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Rockstar Games never officially released the "Definitive Edition" on PSP. The PPSSPP emulator runs the original GTA: Vice City Stories and Liberty City Stories , but not the "Definitive Edition" of San Andreas. However, the modding community has created "Definitive Edition" mods for the original Android/iOS version that run on PPSSPP. Title: GTA SA Definitive Edition on PPSSPP: Is It Real & How to Get the Ultimate Mobile Experience The Dream: Playing the upgraded lighting, modern textures, and GTA V-style controls of GTA San Andreas Definitive Edition on your phone using the PPSSPP emulator. You can’t run the official Definitive Edition (the